Robustness of the charge-ordered phases in IrTe${}_2$ against photoexcitation

Abstract

We present a time-resolved angle-resolved photoelectron spectroscopy study of IrTe${}_2$, which undergoes two first-order structural and charge-ordered phase transitions on cooling below 270 K and below 180 K. The possibility of inducing a phase transition by photoexcitation with near-infrared femtosecond pulses is investigated in the charge-ordered phases. We observe changes of the spectral function occuring within a few hundreds of femtoseconds and persisting up to several picoseconds, which we interpret as a partial photoinduced phase transition (PIPT). The necessary time for photoinducing these spectral changes increases with increasing photoexcitation density and reaches timescales longer than the rise time of the transient electronic temperature. We conclude that the PIPT is driven by a transient increase of the lattice temperature following the energy transfer from the electrons. However, the photoinduced changes of the spectral function are small, which indicates that the low temperature phase is particularly robust against photoexcitation. We suggest that the system might be trapped in an out-of-equilibrium state, for which only a partial structural transition is achieved.

8 pages, 5 figures, accepted for publication in Phys. Rev. B

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• Dynamic short-range correlation in photoinduced disorder phase transitions
• Spatially-resolved electronic structure of stripe domains in IrTe${}_2$ through electronic structure microscopy
• Insensitivity of the striped charge-orders in IrTe${}_2$ to alkali surface doping implies their structural origin
• Break of symmetry at the surface of IrTe${}_2$ upon phase transition measured by X-ray photoelectron diffraction