Local orthorhombicity in the magnetic $C_4$ phase of the hole-doped iron-arsenide superconductor Sr${}_{1-x}$Na${}_x$Fe${}_2$As${}_2$

Abstract

We report temperature-dependent pair distribution function measurements of Sr${}_{1-x}$Na${}_x$Fe${}_2$As${}_2$, an iron-based superconductor system that contains a magnetic phase with reentrant tetragonal symmetry, known as the magnetic $C_4$ phase. Quantitative refinements indicate that the instantaneous local structure in the $C_4$ phase is comprised of fluctuating orthorhombic regions with a length scale of $\sim$2 nm, despite the tetragonal symmetry of the average static structure. Additionally, local orthorhombic fluctuations exist on a similar length scale at temperatures well into the paramagnetic tetragonal phase. These results highlight the exceptionally large nematic susceptibility of iron-based superconductors and have significant implications for the magnetic $C_4$ phase and the neighboring $C_2$ and superconducting phases.