In-situ single-shot diffractive fluence mapping for X-ray free-electron laser pulses

Abstract

Free-electron lasers (FEL) in the extreme ultraviolet (XUV) and X-ray regime opened up the possibility for experiments at high power densities, in particular allowing for fluence-dependent absorption and scattering experiments to reveal non-linear light-matter interactions at ever shorter wavelengths. Findings of such non-linear effects in the XUV and X-ray regime are met with tremendous interest, but prove difficult to understand and model due to the inherent shot-to-shot fluctuations in photon intensity and the often structured, non-Gaussian spatial intensity profile of a focused FEL beam. Presently, the focused beam spot is characterized and optimized separately from the actual experiment. Here, we present the first simultaneous measurement of diffraction signals from solid samples in tandem with the corresponding single-shot spatial fluence distribution on the actual sample. This new in-situ characterization scheme enables fast and direct monitoring and thus control of the sample illumination which ultimately is necessary for a quantitative understanding of non-linear light-matter interaction in X-ray and XUV FEL experiments.

References in corpus (2)

• Femtosecond Diffractive Imaging with a Soft-X-ray Free-Electron Laser
• Creation of X-Ray Transparency of Matter by Stimulated Elastic Forward Scattering

Cited by in corpus (3)

• Laser-induced ultrafast demagnetization and perpendicular magnetic anisotropy reduction in a Co${}_{88}$Tb${}_{12}$ thin film with stripe domains
• XCALIB: a focal spot calibrator for intense X-ray free-electron laser pulses based on the charge state distributions of light atoms
• Simultaneous mapping of the ultrafast time and fluence dependence of the laser-induced insulator-to-metal transition in magnetite