Magnetization process and magnetocaloric effect in geometrically frustrated Ising antiferromagnet and spin ice models on a `Star of David' nanocluster
arXiv:1703.07756 · doi:10.1016/j.jmmm.2017.11.076
Abstract
Magnetic and magnetocaloric properties of geometrically frustrated antiferromagnetic Ising (IA) and ferromagnetic spin ice (SI) models on a nanocluster with a `Star of David' topology, including next-nearest-neighbor (NNN) interactions, are studied by an exact enumeration. In an external field applied in characteristic directions of the respective models, depending on the NNN interaction sign and magnitude, the ground state magnetization of the IA model is found to display up to three intermediate plateaus at fractional values of the saturation magnetization, while the SI model shows only one zero-magnetization plateau and only for the antiferromagnetic NNN coupling. A giant magnetocaloric effect is revealed in the the IA model with the NNN interaction either absent or equal to the nearest-neighbor coupling. The latter is characterized by abrupt isothermal entropy changes at low temperatures and infinitely fast adiabatic temperature variations for specific entropy values in the processes when the magnetic field either vanishes or tends to the critical values related to the magnetization jumps.
13 pages, 8 figures
References in corpus (7)
- Magnetothermal properties of molecule-based materials
- Enhanced magnetocaloric effect in frustrated magnets
- Spin-enhanced magnetocaloric effect in molecular nanomagnets
- Enhanced magnetocaloric effect in frustrated magnetic molecules with icosahedral symmetry
- Giant magnetocaloric effect, magnetization plateaux and jumps of the regular Ising polyhedra
- The Schottky-type specific heat as an indicator of relative degeneracy between ground and first-excited states: the case study of regular Ising polyhedra
- Thermodynamic and magnetocaloric properties of geometrically frustrated Ising nanoclusters
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