Electron spin polarization in strong-field ionization of Xenon atoms

Abstract

As a fundamental property of the electron, the spin plays a decisive role in the electronic structure of matter from solids to molecules and atoms, e.g. causing magnetism. Yet, despite its importance, the spin dynamics of electrons released during the interaction of atoms with strong ultrashort laser pulses has remained unexplored. Here we report on the experimental detection of electron spin polarization by strong-field ionization of Xenon atoms and support our results by theoretical analysis. We found up to 30% spin polarization changing its sign with electron energy. This work opens the new dimension of spin to strong-field physics. It paves the way to production of subfemtosecond spin polarized electron pulses with applications ranging from probing magnetic properties of matter at ultrafast time scales to testing chiral molecular systems with subfemtosecond temporal and sub-Ångström spatial resolution.

9 pages, 3 figures

References in corpus (2)

• Hole dynamics and spin currents after ionization in strong circularly polarized laser fields
• Laser induced ultrafast demagnetization: an \emph{ab-initio} perspective

Cited by in corpus (5)

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• Spin-polarizing interferometric beam splitter for free electrons
• Exit momentum and instantaneous ionization rate of nonadiabatic tunneling ionization in elliptically polarized laser fields
• Accurate in situ Measurement of Ellipticity Based on Sub-cycle Ionization Dynamics
• Spin in Compton scattering with pronounced polarization dynamics