Hierarchy of equations to calculate the linear spectra of molecular aggregates - Time-dependent and frequency domain formulation

Abstract

In a recent publication [J. Chem. Phys. 142, 034115 (2015)] we have derived a hierarchy of coupled differential equations in time domain to calculate the linear optical properties of molecular aggregates. Here we provide details about issues concerning the numerical implementation. In addition we present the corresponding hierarchy in frequency domain.

References in corpus (7)

• Photonics meets excitonics: natural and artificial molecular aggregates
• Hierarchy of stochastic pure states for open quantum system dynamics
• Analytic Representations of Bath Correlation Functions for Ohmic and Superohmic Spectral Densities Using Simple Poles
• Polaron dynamics with a multitude of Davydov D${}_2$ trial states
• Non-Markovian quantum state diffusion for absorption spectra of molecular aggregates
• Non-Markovian Quantum State Diffusion for Temperature-Dependent Linear Spectra of Light Harvesting Aggregates
• Vibronic Lineshapes of PTCDA Oligomers in Helium Nanodroplets

Cited by in corpus (2)

• Flexible scheme to truncate the hierarchy of pure states
• Spectral signatures of the Markovian to Non-Markovian transition in open quantum systems