On Subthreshold Ionization of Helium Droplets, Ejection of He+, and the Role of Anions
arXiv:1611.06769 · doi:10.1039/C4CP03236E
Abstract
The mechanism of ionization of helium droplets has been investigated in numerous reports but one observation has not found a satisfactory explanation: How are ions formed and ejected from undoped droplets at electron energies below the ionization threshold of the free atom? Does this path exist at all? A measurement of the ion yields of and as a function of electron energy, electron emission current, and droplet size reveals that metastable anions play a crucial role in the formation of free at subthreshold energies. The proposed model is testable.