Premelting-Induced Smoothening of the Ice-Vapor Interface
arXiv:1609.01439 · doi:10.1103/PhysRevLett.117.096101
Abstract
We perform computer simulations of the quasiliquid layer of ice formed at the ice-vapor interface close to the ice Ih-liquid-vapor triple point of water. Our study shows that the two distinct surfaces bounding the film behave at small wavelengths as atomically rough and independent ice-water and water-vapor interfaces. For long wavelengths, however, the two surfaces couple, large scale parallel fluctuations are inhibited, and the ice-vapor interface becomes smooth. Our results could help explain the complex morphology of ice crystallites.
postprint plus supplemental material with details on simulation and theory
References in corpus (7)
- Canonical sampling through velocity-rescaling
- Accurate determination of crystal structures based on averaged local bond order parameters
- The thickness of a liquid layer on the free surface of ice as obtained from computer simulation
- Tension and stiffness of the hard sphere crystal-fluid interface
- A study of the ice-water interface using the TIP4P/2005 water model
- Premelting, fluctuations and coarse-graining of water-ice interfaces
- Computer simulation study of surface wave dynamics at the crystal--melt interface
Cited by in corpus (11)
- Intermolecular forces at ice and water interfaces: premelting, surface freezing and regelation
- Structure and fluctuations of the premelted liquid film of ice at the triple point
- Effect of Sodium Chloride Adsorption on the Surface Premelting of Ice
- Structure and water attachment rates of ice in the atmosphere: role of nitrogen
- Premelting and formation of ice due to Casimir-Lifshitz interactions: Impact of improved parameterization for materials
- Premelting layer during ice growth: role of clusters
- Transition dynamics and metastable states during premelting and freezing of ice surfaces
- Is it possible to overheat ice? The activated melting of TIP4P/Ice at solid-vapor coexistence
- Unveiling the Face-Dependent Ice Growth Kinetics: Insights from Molecular Dynamics on the Basal and Prism Surfaces
- Binding potentials for vapour nanobubbles on surfaces using density functional theory
- The Key Physics of Ice Premelting