Probing strongly hybrid nuclear-electronic states in a model quantum ferromagnet

Abstract

We present direct local-probe evidence for strongly hybridized nuclear-electronic spin states of an Ising ferromagnet LiHoF${}_4$ in a transverse magnetic field. The nuclear-electronic states are addressed via a magnetic resonance in the GHz frequency range using coplanar resonators and a vector network analyzer. The magnetic resonance spectrum is successfully traced over the entire field-temperature phase diagram, which is remarkably well reproduced by mean-field calculations. Our method can be directly applied to a broad class of materials containing rare-earth ions for probing the substantially mixed nature of the nuclear and electronic moments.

arXiv comment6 pages, 5 figures

References in corpus (14)

• Concentrating Partial Entanglement by Local Operations
• Nuclear spin driven quantum relaxation in LiY_0.998Ho_0.002F_4
• Quantum Phase Transition of a Magnet in a Spin Bath
• Initializing, manipulating and storing quantum information with bismuth dopants in silicon
• Quantum and Classical Glass Transitions in $LiH{o}_x{Y}_{1-x}{F}_4$
• Ferromagnet in a continuously tuneable random field
• Significance of the Hyperfine Interactions in the Phase Diagram of $\mathrm{LiH}{\mathrm{o}}_{\mathrm{x}}{\mathrm{Y}}_{1-\mathrm{x}}{\mathrm{F}}_4$
• Quantum control of hybrid nuclear-electronic qubits
• The quantum dynamics of atomic magnets, co-tunneling and dipolar-biased tunneling
• The low-$T$ phase diagram of $\mathrm{LiH}{\mathrm{o}}_{\mathrm{x}}{\mathrm{Y}}_{1-\mathrm{x}}{\mathrm{F}}_4$
• Neutron spectroscopic study of crystal-field excitations and the effect of the crystal field on dipolar magnetism in Li$R$F${}_4$ ($R$ = Gd, Ho, Er, Tm, and Yb)
• A field trip through spin ice
• Dimensional Reduction in Quantum Dipolar Antiferromagnets
• Non-equilibrium hysteresis and spin relaxation in the mixed-anisotropy dipolar coupled spin-glass LiHo${}_{0.5}$Er${}_{0.5}$F${}_4$

Cited by in corpus (7)

• Direct Observation of Collective Electronuclear Modes About a Quantum Critical Point
• Theory of magnon-polaritons in quantum Ising materials
• Limits to magnetic quantum criticality from nuclear spins
• Microscopic spin Hamiltonian for a dipolar-Heisenberg magnet LiGdF4 from EPR measurements
• Partitioned Density Matrices and Entanglement Correlators
• Cavity-Magnon-Polariton spectroscopy of strongly hybridized electro-nuclear spin excitations in LiHoF4
• Thermodynamics of a Quantum Ising system coupled to a spin bath: Zero Temperature Results