paper

Low-Energy Excitations and Ground State Selection in Quantum Breathing Pyrochlore Antiferromagnet BaYbZnO

arXiv:1605.08544 · doi:10.1103/PhysRevB.93.220407

Abstract

We study low energy excitations in the quantum breathing pyrochlore antiferromagnet BaYbZnO by combination of inelastic neutron scattering (INS) and thermodynamical properties measurements. The INS spectra are quantitatively explained by spin-1/2 single-tetrahedron model having anisotropy and Dzyaloshinskii-Moriya interaction. This model has a two-fold degeneracy of the lowest-energy state per tetrahedron and well reproduces the magnetization curve at 0.5 K and heat capacity above 1.5 K. At lower temperatures, however, we observe a broad maximum in the heat capacity around 63 mK, demonstrating that a unique quantum ground state is selected due to extra perturbations with energy scale smaller than the instrumental resolution of INS.

5 pages 3 figures, Phys. Rev. B rapid communication in press