Angle-resolved spectroscopy study of Ni-based superconductor SrNi${}_2$As${}_2$

Abstract

We performed an angle-resolved photoemission spectroscopy study of the Ni-based superconductor SrNi${}_2$As${}_2$. Electron and hole Fermi surface pockets are observed, but their different shapes and sizes lead to very poor nesting conditions. The experimental electronic band structure of SrNi${}_2$As${}_2$ is in good agreement with first-principles calculations after a slight renormalization (by a factor 1.1), confirming the picture of Hund's exchange-dominated electronic correlations decreasing with increasing filling of the $3d$ shell in the Fe-, Co- and Ni-based compounds. These findings emphasize the importance of Hund's coupling and $3d$-orbital filling as key tuning parameters of electronic correlations in transition metal pnictides.

6 pages, 5 figures. New title. Data and discussions on SrNi2P2 removed