Uniaxial pressure induced half-metallic ferromagnetic phase transition in LaMnO${}_3$

Abstract

We use first-principles theory to predict that the application of uniaxial compressive strain leads to a transition from an antiferromagnetic insulator to a ferromagnetic half-metal phase in LaMnO${}_3$. We identify the Q2 Jahn-Teller mode as the primary mechanism that drives the transition, indicating that this mode can be used to tune the lattice, charge, and spin coupling. Applying $\simeq$ 6 GPa of uniaxial pressure along the [010] direction activates the transition to a half-metallic $\text{pseudo-cubic}$ state. The half-metallicity opens the possibility of producing colossal magnetoresistance in the stoichiometric LaMnO${}_3$ compound at significantly lower pressure compared to recently observed investigations using hydrostatic pressure.