Structural Domain Switching by Magnetic Fields in RAl${}_3$C${}_3$ (R=Rare Earth)

Abstract

Hexagonal-to-orthorhombic structural transitions in RAl${}_3$C${}_3$ have been studied by X-ray diffraction for R=Yb, Tm, Er, Dy, and Lu. We report how orthorhombic domains are controlled by adjusting external magnetic fields. It is shown that orthorhombic domains in RAl${}_3$C${}_3$ can be aligned by the field when the R ion is magnetic. It is also shown that a single-domain state can be switched to another single-domain state by the field even in paramagnetic states with small induced moments. For R=Lu, however, it was not possible to change the multidomain state by a field of up to 70 kOe. We discuss that domain selection and switching are caused by magnetic anisotropies in the orthorhombic phase of RAl${}_3$C${}_3$. We also propose an idea to explain the field-induced antiferromagnetism revealed by Khalyavin et al. [Phys. Rev. B \textbf{87}, 220406 (2013)].

8 pages, 10 figures, 1 table, accepted in J. Phys. Soc. Jpn

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