Complete Photoionization Experiments via Ultrafast Coherent Control with Polarization Multiplexing II: Numerics & Analysis Methodologies

Abstract

The feasibility of complete photoionization experiments, in which the full set of photoionization matrix elements are determined, using multiphoton ionization schemes with polarization-shaped pulses has recently been demonstrated [Hockett et. al., Phys. Rev. Lett. 112, 223001 (2014)]. Here we extend on our previous work to discuss further details of the numerics and analysis methodology utilised, and compare the results directly to new tomographic photoelectron measurements, which provide a more sensitive test of the validity of the results. In so doing we discuss in detail the physics of the photoionziation process, and suggest various avenues and prospects for this coherent multiplexing methodology.

References in corpus (3)

• Momentum space tomographic imaging of photoelectrons
• Complete photoionization experiments via ultra-fast coherent control with polarization-multiplexing
• Maximum information photoelectron metrology

Cited by in corpus (6)

• Bootstrapping to the Molecular Frame with Time-domain Photoionization Interferometry
• Angle-resolved RABBIT: theory and numerics
• Maximum information photoelectron metrology
• Coherent Control of Photoelectron Wavepacket Angular Interferograms
• Topical Review: Extracting Molecular Frame Photoionization Dynamics from Experimental Data
• Multiphoton ionization with three-dimensional light fields