Unusual Shubnikov-de Haas oscillations in BiTeCl

Abstract

We report measurements of Shubnikov-de Haas (SdH) oscillations in single crystals of BiTeCl at magnetic fields up to 31 T and at temperatures as low as 0.4 K. Two oscillation frequencies were resolved at the lowest temperatures, $F_1=65\pm 4$ Tesla and $F_2=156\pm 5$ Tesla. We also measured the infrared optical reflectance $\left(\mathcal{R}(\omega )\right)$ and Hall effect; we propose that the two frequencies correspond respectively to the inner and outer Fermi sheets of the Rashba spin-split bulk conduction band. The bulk carrier concentration was $n_e\approx 1\times 10^{19}$ cm${}^{-3}$ and the effective masses $m_1^{\ast }=0.20m_0$ for the inner and $m_2^{\ast }=0.27m_0$ for the outer sheet. Surprisingly, despite its low effective mass, we found that the amplitude of $F_2$ is very rapidly suppressed with increasing temperature, being almost undetectable above $T\approx 4$ K.

References in corpus (12)

• Topological Insulators
• Topological Insulators with Inversion Symmetry
• Fermi Surface Topological Invariants for Time Reversal Invariant Superconductors
• Emergence of non-centrosymmetric topological insulating phase in BiTeI under pressure
• Ideal two-dimensional electron systems with a giant Rashba-type spin splitting in real materials: surfaces of bismuth tellurohalides
• Giant ambipolar Rashba effect in a semiconductor: BiTeI
• Signatures of a Pressure-Induced Topological Quantum Phase Transition in BiTeI
• Surface and bulk Fermiology and band dispersion in non-centrosymmetric BiTeI
• Infrared and Raman spectroscopy measurements of a transition in the crystal structure and a closing of the energy gap of BiTeI under pressure
• Quantum oscillations and optical conductivity in Rashba spin-splitting BiTeI
• Optical properties of BiTeBr and BiTeCl
• Transport evidence of robust topological surface state in BiTeCl single crystals, the first strong inversion asymmetric topological insulator

Cited by in corpus (8)

• Use of X-ray scattering functions in Kramers-Kronig analysis of reflectance
• Observation of topological transition of Fermi surface from a spindle-torus to a torus in large bulk Rashba spin-split BiTeCl
• Large Enhancement of Thermoelectric Efficiency Due to a Pressure-Induced Lifshitz Transition in SnSe
• Temperature dependence of the bulk Rashba splitting in the bismuth tellurohalides
• Superconductivity in Dense Rashba Semiconductor BiTeCl
• Magnetic susceptibility of topological semimetals
• Unusual magnetoresistance oscillations in preferentially oriented p-type polycrystalline ZrTe5
• Evolution of the Fermi surface of BiTeCl with pressure