Control of populations of two-level systems by a single resonant laser pulse

Abstract

We present a simple approach allowing to obtain analytical expressions for laser pulses that can drive a two-level system in an arbitrarily chosen way. The proposed scheme relates every desired population-evolution path to a single resonant laser pulse. It allows to drive the system from any initial superposition of the two states to a final state having the desired distribution of the populations. We exemplify the scheme with a concrete example, where the system is driven from a non-stationary superposition of states to one of its eigenstates. We argue that the proposed approach may have interesting applications for designing pulses that can control ultrafast charge-migration processes in molecules. Although focused on laser driven population control, the results obtained are general and could be applied for designing other types of control fields.

References in corpus (1)

• Radiation Generated by Charge Migration Following Ionization

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