Nonlinear response functions in an exponential trap model

Abstract

The nonlinear response to an oscillating field is calculated for a kinetic trap model with an exponential density of states and the results are compared to those for the model with a Gaussian density of states. The calculations are limited to the high temperature phase of the model. It is found that the results are qualitatively different only in a temperature range near the glass transition temperature $T_0$ of the exponential model. While for the Gaussian model the choice of the dynamical variable that couples to the field has no impact on the shape of the linear response, this is different for the exponential model. Here, it is found that also the relaxation time strongly depends on the variable chosen. Furthermore, the modulus of the frequency dependent third-order response shows either a peak or exhibits a monotonuous decay from a finite low-frequency limit to a vanishing response at high frequencies depending on the dynamical variable. For variables that give rise to a peak in the modulus it is found that its height either increases or decreases as a function of temperature, again depending on the details of the choice of the variable. The peak value of the modulus shows a scaling behavior near $T_0$. It is found that for some variables the low-frequency limit of the cubic response diverges at the glass transition temperature and also at a further temperature determined by the particular variable. A recently proposed approximation that relates the cubic response to a four-time correlation function does not give reliable results due to a wrong estimate of the low-frequency limit of the response.

11 pages, 7 figures

References in corpus (15)

• Direct experimental evidence of a growing length scale accompanying the glass transition
• Models of traps and glass phenomenology
• What do we learn from the shape of the dynamical susceptibility of glass-formers?
• Spontaneous and induced dynamic fluctuations in glass-formers I: General results and dependence on ensemble and dynamics
• Dynamic heterogeneity in amorphous materials
• Spontaneous and induced dynamic correlations in glass-formers II: Model calculations and comparison to numerical simulations
• Non-linear susceptibility in glassy systems: a probe for cooperative dynamical length scales
• Evidence of growing spatial correlations at the glass transition from nonlinear response experiments
• Observable-dependence of fluctuation-dissipation relations and effective temperatures
• Nonlinear response theory for Markov processes: Simple models for glassy relaxation
• Dynamical Heterogeneity and Nonlinear Susceptibility in Short-Ranged Attractive Supercooled Liquids
• Aging effects manifested in the potential energy landscape of a model glass former
• Memory effects in the relaxation of the Gaussian trap model
• Higher-order correlation functions and nonlinear response functions in a Gaussian trap model
• Out-of-equilibrium dynamics in a gaussian trap model

Cited by in corpus (1)

• Nonlinear response theory for Markov processes IV: The asymmetric double well potential model revisited