Optical-phonon resonances with saddle-point excitons in twisted-bilayer graphene

Abstract

Twisted-bilayer graphene (tBLG) exhibits van Hove singularities in the density of states that can be tuned by changing the twisting angle $\theta$. A $\theta$-defined tBLG has been produced and characterized with optical reflectivity and resonance Raman scattering. The $\theta$-engineered optical response is shown to be consistent with persistent saddle-point excitons. Separate resonances with Stokes and anti-Stokes Raman scattering components can be achieved due to the sharpness of the two-dimensional saddle-point excitons, similar to what has been previously observed for one-dimensional carbon nanotubes. The excitation power dependence for the Stokes and anti-Stokes emissions indicate that the two processes are correlated and that they share the same phonon.

5 pages, 6 figures

References in corpus (2)

• Flat Bands in Slightly Twisted Bilayer Graphene
• Raman-scattering study of the phonon dispersion in twisted bi-layer graphene

Cited by in corpus (5)

• Flat-band optical phonons in twisted bilayer graphene
• Ideal pairing of the Stokes and anti-Stokes photons in the Raman process
• Excitonic effects in twisted bilayer graphene
• Emergent broadband polarization entanglement from electronic and phononic Stokes-anti-Stokes indistinguishability
• Exciton lasing in carbon nanotubes below the population inversion threshold via phonon-mediated stimulated emission