Long-wavelength fluctuations lead to a model of the glass crossover
arXiv:1405.6557 · doi:10.1209/0295-5075/106/56003
Abstract
The effect of long wavelength fluctuations on the Mode-Coupling-Theory (MCT) dynamical singularity at in the regime is studied by means of the standard field-theoretical procedure for a genuine second-order phase transition. The resulting perturbative loop expansion can be resummed leading to an extension of the MCT equation for the critical correlator with local random fluctuations of the separation parameter. The corresponding model explains both qualitatively and quantitatively why the MCT dynamical singularity is transformed into a crossover from relaxational to activated dynamics. Dynamical Heterogeneities emerge naturally as the ergodicity-restoring mechanism instead of {\it ad hoc} hopping processes.
arXiv commentAccepted for publication on EPL, based on talk given at 7 IDMRCS (arxiv:1307.4303)
References in corpus (20)
- Dynamical heterogeneities in a supercooled Lennard-Jones liquid
- Inhomogeneous Mode-Coupling Theory and Growing Dynamic Length in Supercooled Liquids
- Spontaneous and induced dynamic fluctuations in glass-formers I: General results and dependence on ensemble and dynamics
- Corresponding States of Structural Glass Formers
- How does the relaxation of a supercooled liquid depend on its microscopic dynamics?
- Spontaneous and induced dynamic correlations in glass-formers II: Model calculations and comparison to numerical simulations
- The Debye-Waller factor of liquid silica: Theory and simulation
- Structural relaxation of polydisperse hard spheres: comparison of the mode-coupling theory to a Langevin dynamics simulation
- Field Theory of Fluctuations in Glasses
- Cooperativity Beyond Caging: Generalized Mode Coupling Theory
- Connections of activated hopping processes with the breakdown of the Stokes-Einstein relation and with aspects of dynamical heterogeneities
- Quantitative field theory of the glass transition
- Universal and non-universal features of glassy relaxation in propylene carbonate
- On the critical slowing down exponents of mode coupling theory
- Critical Dynamics in Glassy Systems
- Dynamic glass transition: bridging the gap between mode-coupling theory and the replica approach
- Characterizing dynamic length scales in glass-forming liquids
- Crossover behavior and multi-step relaxation in a schematic model of the cut-off glass transition
- Super-Cooled Liquids: Equivalence between Mode-Coupling Theory and Replica Approach
- A note on weakly discontinuous dynamical transitions
Cited by in corpus (26)
- Particle jumps in structural glasses
- Spinodals with Disorder: from Avalanches in Random Magnets to Glassy Dynamics
- A simple theory for the dynamics of mean-field-like models of glass-forming fluids
- Qualitative Features at the Glass Crossover
- Quantitative approximation schemes for glasses
- Non-linear dynamic response of glass-forming liquids to random pinning
- Dynamical Landau Theory of the Glass Crossover
- Path Integral Approach Unveils the Role of Complex Energy Landscape for Activated Dynamics of Glassy Systems
- Solvable Models of Supercooled Liquids in Three Dimensions
- Random-field Ising model criticality in a glass-forming liquid
- Spatial correlations of elementary relaxation events in glass-forming liquids
- The fate of the bootstrap percolation hybrid critical point in finite dimension
- Non-monotonic dynamic correlations beneath the surface of glass-forming liquids
- From sub-aging to hyper-aging in structural glasses
- The Fredrickson-Andersen model with random pinning on Bethe lattices and its MCT transitions
- Unveiling the anatomy of mode-coupling theory
- Theory of heterogeneous viscoelasticity
- The Glass Crossover from Mean-Field Spin-Glasses to Supercooled Liquids
- Continuous time random walk concepts applied to extended mode coupling theory: A study of the Stokes-Einstein breakdown
- Thermodynamics of the Fredrickson-Andersen Model on the Bethe Lattice
- Theory of Kinetically-Constrained-Models Dynamics
- Logarithmic critical slowing down in complex systems: from statics to dynamics
- Theory of the -Relaxation Beyond Mode-Coupling Theory: A Microscopic Treatment
- Microscopic Theory of a Fluctuation-Induced Dynamical Crossover in Supercooled Liquids
- An alternative, dynamic density functional-like theory for time-dependent density fluctuations in glass-forming fluids
- Full replica symmetry breaking in p-spin-glass-like systems