Large-amplitude spin oscillations triggered by nonequilibrium strongly correlated $t_{2g}$ electrons

Abstract

Laser-induced ultrafast (fs) magnetization experiments in antiferromagnets have recently attracted large attention, paving the road for inherently fast spin dynamics in the THz regime without invoking stray fields. The technical importance is emphasized by the rising new research field of antiferromagnetic (AFM) spintronics, where superexchange-dominated strongly correlated compounds provide an interesting materials playground. An intriguing question is whether the Coulomb interaction may be a key to control AFM order on ultrafast time scales. Therefore, we study (de)magnetization processes in a time-dependent multiorbital Hubbard model, focusing on $t_{2g}$ electrons in a wider doping range. Depending on filling, we reveal large-amplitude spin oscillations via interaction quenches from the antiferromagnetic or paramagnetic state. Nonequilibrium ultrafast spin-orientation effects in prominent correlated transition-metal oxides are therefrom predicted.

arXiv comment6 pages and 3 pages Appendix, 7 figures and 1 figure in Appendix

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• Hund's coupling driven photo-carrier relaxation in the two-band Mott insulator
• Rigorous symmetry adaptation of multiorbital rotationally invariant slave-boson theory with application to Hund's rules physics
• Versatile Approach to the Spin Dynamics in Correlated Electron Systems