Nodal "ground states" and orbital textures in semiconductor quantum dots

Abstract

Conventional understanding implies that the ground state of a nonmagnetic quantum mechanical system should be nodeless. While this notion also provides a valuable guidance in understanding the ordering of energy levels in semiconductor nanostructures, there are reports that $\text{nodal}$ ground states for holes are possible. However, the existence of such nodal states has been debated and even viewed merely as an artifact of a $\mathbf{k}\cdot \mathbf{p}$ model. Using complementary approaches of both $\mathbf{k}\cdot \mathbf{p}$ and tight-binding models, further supported by an effective Hamiltonian for a continuum model, we reveal that the nodal ground states in quantum dots are not limited to a specific approach. Remarkably, the emergence of the nodal hole states at the top of the valence band can be attributed to the formation of the orbital vortex textures through competition between the hole kinetic energy and the coupling to the conduction band states. We suggest an experimental test for our predictions of the reversed energy ordering and the existence of nodal ground states. We discuss how our findings and the studies of orbital textures could be also relevant for other materials systems.

19 pages, 14 figures, submitted to PRB, identical to v2 with pdf compatibility issue of figures resolved

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Cited by in corpus (6)

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• Wurtzite spin lasers
• Time-resolved magnetophotoluminescence studies of magnetic polaron dynamics in type-II quantum dots
• Ground state of an exciton in a three-dimensional parabolic quantum dot: convergent perturbative calculation
• Emergent bright excitons with Rashba spin-orbit coupling in atomic monolayers
• Magnetic ordering in quantum dots: Open vs. closed shells