Combined action of the bound-electron nonlinearity and the tunnel-ionization current in low-order harmonic generation in noble gases
arXiv:1311.1351 · doi:10.1364/OE.21.025582
Abstract
We study numerically low-order harmonic generation in noble gases pumped by intense femtosecond laser pulses in the tunneling ionization regime. We analyze the influence of the phase-mismatching on this process, caused by the generated plasma, and study in dependence on the pump intensity the origin of harmonic generation arising either from the bound-electron nonlinearity or the tunnel-ionization current. It is shown that in argon the optimum pump intensity of about 100 TW/cm leads to the maximum efficiency, where the main contribution to low-order harmonics originates from the bound-electron third and fifth order susceptibilities, while for intensities higher than 300 TW/cm the tunnel-ionization current plays the dominant role. Besides, we predict that VUV pulses at 133 nm can be generated with relatively high efficiency of about by 400 nm pump pulses.
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