High-order harmonic generation from field-distorted orbitals

Abstract

We investigate the effect on high-order harmonic generation of the distortion of molecular orbitals by the driving laser field. Calculations for high-order harmonic generation including orbital distortion are performed for N2. Our results allow us to suggest that field-distortion is the reason why the two-center interference minimum has never been observed experimentally in N2. We propose experimental parameters which should allow an observation of the two-center interference minimum.

References in corpus (5)

• Phase-Matched Generation of Coherent Soft-X-Rays
• Shaped-pulse optimisation of coherent soft-x-rays
• Intensity dependence of multiple orbital contributions and shape resonance in high-order harmonic generation of aligned N${}_2$ molecules}
• Molecular Orbital Tomography using Short Laser Pulses
• Molecular Recollision Interferometry in High Harmonic Generation

Cited by in corpus (4)

• Dynamic orbitals in high-harmonic generation from CO molecules
• Dynamical distortions of structural signatures in molecular High Harmonic Spectroscopy
• Semi-Classical Wavefunction Perspective to High-Harmonic Generation
• Attosecond Molecular Spectroscopy and Dynamics