Decorrelation of the static and dynamic length scales in hard-sphere glass-formers
arXiv:1211.4821 · doi:10.1103/PhysRevE.87.042305
Abstract
We show that in the equilibrium phase of glass-forming hard-sphere fluids in three dimensions, the static length scales tentatively associated with the dynamical slowdown and the dynamical length characterizing spatial heterogeneities in the dynamics unambiguously decorrelate. The former grow at a much slower rate than the latter when density increases. This observation is valid for the dynamical range that is accessible to computer simulations, which roughly corresponds to that of colloidal experiments. We also find that in this same range, no one-to-one correspondence between relaxation time and point-to-set correlation length exists. These results point to the coexistence of several relaxation mechanisms in the accessible dynamical regime of three-dimensional hard-sphere glass formers.
8 pages, 7 figures
References in corpus (17)
- Packing Hyperspheres in High-Dimensional Euclidean Spaces
- Roles of icosahedral and crystal-like order in hard spheres glass transition
- Growing length and time scales in glass forming liquids
- Spontaneous and induced dynamic fluctuations in glass-formers I: General results and dependence on ensemble and dynamics
- Rigorous Inequalities between Length and Time Scales in Glassy Systems
- The glass transition of dense fluids of hard and compressible spheres
- Understanding fragility in supercooled Lennard-Jones mixtures. I. Locally preferred structures
- Identification of long-lived clusters and their link to slow dynamics in a model glass former
- Alpha-Relaxation Processes in Binary Hard-Sphere Mixtures
- Locally preferred structures and many-body static correlations in viscous liquids
- Mixing effects for the structural relaxation in binary hard-sphere liquids
- Finite size effects in the dynamics of glass-forming liquids
- Dimensional Study of the Caging Order Parameter at the Glass Transition
- Multiple length and time scales of dynamic heterogeneities in model glass-forming liquids: A systematic analysis of multi-point and multi-time correlations
- Tuning the fragility of a glassforming liquid by curving space
- Characterizing order in amorphous systems
- Geometrical Frustration and Static Correlations in Hard-Sphere Glass Formers
Cited by in corpus (21)
- The role of local structure in dynamical arrest
- Direct measurements of growing amorphous order and non-monotonic dynamic correlations in a colloidal glass-former
- Thirty milliseconds in the life of a supercooled liquid
- Growing Dynamical Facilitation on Approaching the Random Pinning Colloidal Glass Transition
- Strong geometric frustration in model glassformers
- Deconstructing the glass transition through critical experiments on colloids
- Experimental evidence of a crossover between cooperative relaxation and liquid growth dynamics
- Dynamical facilitation governs glassy dynamics in suspensions of colloidal ellipsoids
- Roles of liquid structural ordering in glass transition, crystallization, and water's anomalies
- Block Analysis for the Calculation of Dynamic and Static Length Scales in Glass-Forming Liquids
- Dynamic heterogeneity at the experimental glass transition predicted by transferable machine learning
- Collective relaxation dynamics in a three-dimensional lattice glass model
- Simple physics of the partly pinned fluid systems
- Enhanced diffusion in finite-size simulations of a fragile diatomic glass former
- Glassy phases of the Gaussian Core Model
- Creating equilibrium glassy states via random particle bonding
- The potential energy landscape and inherent dynamics of a hard-sphere fluid
- Characterising the slow dynamics of the swap Monte Carlo algorithm
- Computational Methods toward Ultrastable Glasses
- Free-energy functional of instantaneous correlation field in liquids: field-theoretic derivation of the closures
- Configurational Entropy of Self Propelled Glass Formers