paper

Frustrated magnets and quantum paramagnetic phases at finite temperature

arXiv:1204.2559 · doi:10.1103/PhysRevB.86.100402

Abstract

We develop a general framework, which combines exact diagonalization in small clusters with a density matrix variational principle, to study frustrated magnets at finite temperature. This thermodynamic hierarchical mean-field technique is used to determine the phase diagram and magnetization process of the three-dimensional spin-1/2 - antiferromagnet on a stacked square lattice. Its non-magnetic phase exhibits a thermal crossover from a quantum to a classical paramagnet at a temperature which can be extracted from thermodynamic measurements. At low temperature an applied magnetic field stabilizes, through order-by-disorder, a variety of phases with non-trivial spin textures and a magnetization plateau at half-saturation which continuously disappears at . Our results are relevant for frustrated vanadium oxides.

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