Kinetic Energy Release in Fragmentation Processes following Electron Emission: A time dependent approach
arXiv:1202.1704 · doi:10.1063/1.3694536
Abstract
A time-dependent approach for the kinetic energy release (KER) spectrum is developed for a fragmentation of a diatomic molecule after an electronic decay process, e.g. Auger process. It allows one to simulate the time-resolved spectra and provides more insight into the molecular dynamics than the time-independent approach. Detailed analysis of the time-resolved emitted electron and KER spectra sheds light on the interrelation between wave packet dynamics and spectra.
This article has been modified and the newest version can be found in (J. Chem. Phys. 136, 114111 (2012)) at (http://link.aip.org/link/?JCP/136/114111). Copyright (2012) American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics