paper

Plasmon enhanced upconversion luminescence near gold nanoparticles - Simulation and analysis of the interactions

arXiv:1110.6072 · doi:10.1364/OE.20.000271

Abstract

We investigate plasmon resonances in gold nanoparticles to enhance the quantum yield of upconverting materials. For this purpose, we use a rate equation model that describes the upconversion of trivalent erbium based upconverters. Changes of the optical field acting on the upconverter and the changes to the transition probabilities of the upconverter in the proximity of a gold nanoparticle are calculated using Mie theory and exact electrodynamic theory respectively. With this data, the influence on the luminescence of the upconverter is determined using the rate equation model. The results show that upconversion luminescence can be increased in the proximity of a spherical gold nanoparticle due to the change in the optical field and the modification of the transition rates.

This paper was published in Optics Express and is made available as an electronic reprint with the permission of OSA. The paper can be found at the following on the OSA website: http://www.opticsinfobase.org/oe/abstract.cfm?uri=oe-20-1-271. Systematic or multiple reproduction or distribution to multiple locations via electronic or other means is prohibited and is subject to penalties under law

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