Shape of spin density wave versus temperature in AFe2As2 (A=Ca, Ba, Eu): A Mössbauer study
arXiv:1101.3225 · doi:10.1103/PhysRevB.83.134410
Abstract
Parent compounds AFe2As2 (A=Ca, Ba, Eu) of the 122 family of the iron-based superconductors have been studied by 57Fe Moessbauer spectroscopy in the temperature range 4.2 K - ~300 K. Spin density waves (SDW) have been found with some confidence. They are either incommensurate with the lattice period or the ratio of the respective periods is far away from ratio of small integers. SDW shape is very unconventional i.e. differs from the sinusoidal shape. Magnetic order starts with lowered temperature as narrow sheets of the significant electron spin density separated by areas with very small spin density. Magnetic sheets are likely to be ordered in the alternate anti-ferromagnetic fashion as the material as whole behaves similarly to collinear anti-ferromagnet. Further lowering of temperature simply expands sheet thickness leading to the near triangular SDW. Finally, sheets fill the whole available space and almost rectangular shape of SDW is reached. Substantial maximum amplitude of SDW appears at the temperature just below the magnetic onset temperature, and this maximum amplitude increases slightly with lowering temperature. The square root from the mean squared hyperfine field behaves versus temperature according to the universality class (1, 2), i.e., with the electronic spin space having dimensionality equal unity and the real space having dimensionality equal two. The more or less pronounced tail above transition temperature due to the development of incoherent SDW is seen.
19 pages, 6 figures, 2 tables, accepted in Phys. Rev. B
References in corpus (13)
- Spin density wave anomaly at 140 K in the ternary iron arsenide BaFe2As2
- Commensurate Spin Density Wave in LaOFeAs: A Local Probe Study
- Structural and magnetic phase transitions in the ternary iron arsenides SrFe2As2 and EuFe2As2
- Commensurate Itinerant Antiferromagnetism in BaFe2As2: 75As-NMR Studies on a Self-Flux Grown Single Crystal
- Synthesis and Properties of CaFeAs Single Crystals
- Spin Ordering in LaOFeAs and Its Suppression in Superconductor LaO0.89F0.11FeAs Probed by Mössbauer Spectroscopy
- Competition of magnetism and superconductivity in underdoped (Ba1-xKx)Fe2As2
- Synthesis, crystal structure and spin-density-wave anomaly of the iron arsenide-fluoride SrFeAsF
- Anisotropic magnetic and superconducting properties of pure and Co-doped CaFeAs single crystals
- Neutron scattering investigation of the magnetic order in single crystalline BaFe2As2
- Interplay between superconductivity and magnetism in K-doped EuFe2As2
- Low energy spin dynamics in the antiferromagnetic phase of CaFe2As2
- 75As NMR study of the ternary iron arsenide BaFe2As2