Nonlocal Landau theory of the magnetic phase diagram of highly frustrated magnetoelectric CuFeO${}_2$

Abstract

A nonlocal Landau-type free energy functional of the spin density is developed to model the large variety of magnetic states which occur in the magnetic field-temperature phase diagram of magnetoelectric CuFeO${}_2$. Competition among long-range quadratic exchange, biquadratic anti-symmetric exchange, and trigonal anisotropy terms, consistent with the high-temperature rhombohedral R$\bar{3}$m crystal symmetry, are shown to all play important roles in stabilizing the unusual combination of commensurate and incommensurate spin structures in this highly frustrated triangular antiferromagnet. It is argued that strong magnetoelastic coupling is largely responsible for the nonlocal nature of the free energy. A key feature of the analysis is that an electric polarization is induced by a canting of the non-collinear incommensurate spin structure. Application of the model to ordered spin states in the triangular antiferromagnets MnBr${}_2$ and NaFeO${}_2$ is also discussed.

arXiv comment20 pages, 2 figures

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• A model of magnetic order in hexagonal HoMnO3
• High-Pressure Suppression of Long Range Magnetic Order in the Triangular Lattice Antiferromagnet CuFeO2
• Tracking a hysteretic and disorder-broadened phase transition via the electromagnon response in improper ferroelectrics