Probing the photonic local density of states with electron energy loss spectroscopy
arXiv:0710.5553 · doi:10.1103/PhysRevLett.100.106804
Abstract
Electron energy-loss spectroscopy (EELS) performed in transmission electron microscopes is shown to directly render the photonic local density of states (LDOS) with unprecedented spatial resolution, currently below the nanometer. Two special cases are discussed in detail: (i) 2D photonic structures with the electrons moving along the translational axis of symmetry and (ii) quasi-planar plasmonic structures under normal incidence. Nanophotonics in general and plasmonics in particular should benefit from these results connecting the unmatched spatial resolution of EELS with its ability to probe basic optical properties like the photonic LDOS.
4 pages, 2 figures
Cited by in corpus (67)
- Optical excitations in electron microscopy
- Electron Beam Spectroscopy for Nanophotonics
- Simulating electron energy loss spectroscopy with the MNPBEM toolbox
- Controlling free electrons with optical whispering-gallery modes
- Surface plasmon Fourier optics
- Integrated photonics enables continuous-beam electron phase modulation
- 3D optical manipulation of a single electron spin
- Probing the symmetry of the potential of localized surface plasmon resonances with phase-shaped electron beams
- Probing Quantum Optical Excitations with Fast Electrons
- Electrically driven photon emission from individual atomic defects in monolayer WS2
- Exciton mapping at subwavelength scales in two-dimensional materials
- Extremely confined gap surface plasmon modes excited by electrons
- turboEELS -- A code for the simulation of the electron energy loss and inelastic X-ray scattering spectra using the Liouville-Lanczos approach to time-dependent density-functional perturbation theory
- Characterizing localized surface plasmons using electron energy-loss spectroscopy
- Tuning the electromagnetic local density of states in graphene-covered systems via strong coupling with graphene plasmons
- Roadmap for Photonics with 2D Materials
- Interaction of electron beams with optical nanostructures and metamaterials: From coherent photon sources towards shaping the wave function
- Towards atomic-resolution quantum measurements with coherently-shaped free electrons
- Three dimensional vectorial imaging of surface phonons
- Tunable terahertz radiation from graphene induced by moving electrons
- Tomography of particle plasmon fields from electron energy loss spectroscopy
- Multimodal Plasmonics in Fused Colloidal Networks
- Spontaneous and Stimulated Electron-Photon Interactions in Nanoscale Plasmonic Near Fields
- Nonlocal quasinormal modes for arbitrarily shaped three-dimensional plasmonic resonators
- Purcell factor for point-like dipolar emitter coupling to 2D-plasmonic waveguides
- Control of quantum electrodynamical processes by shaping electron wavepackets
- Tailored nanoscale plasmon-enhanced vibrational electron spectroscopy
- Vibrational surface EELS probes confined Fuchs-Kliewer modes
- Probing the Electrical Switching of a Memristive Optical Antenna by STEM EELS
- Momentum-resolved Electron Energy Loss Spectroscopy for Mapping the Photonic Density of States
- Regularized quasinormal modes for plasmonic resonators and open cavities
- Optical polarization analogue in free electrons beams
- eV electron spectromicroscopy using free-space light
- Interaction of edge exciton polaritons with engineered defects in the van der Waals material Bi2Se3
- Ultrafast Topological Engineering in Metamaterials
- Magnetically Activated Rotational Vacuum Friction
- Time-correlated electron and photon counting microscopy
- Free-Electron Ramsey-Type Interferometry for Enhanced Amplitude and Phase imaging of Nearfields
- Using Electron Energy-Loss Spectroscopy to Measure Nanoscale Electronic and Vibrational Dynamics in a TEM
- Disentangling cathodoluminescence spectra in nanophotonics: particle eigenmodes vs transition radiation
- Influence of experimental conditions on localized surface plasmon resonances measurement by electron energy loss spectroscopy
- Toward Optimum Coupling between Free Electrons and Confined Optical Modes
- Probing and steering bulk and surface phonon polaritons in uniaxial materials using fast electrons: hexagonal boron nitride
- Aluminum Cayley trees as scalable, broadband, multi-resonant optical antennas
- Quasinormal mode theory and modelling of electron energy loss spectroscopy for plasmonic nanostructures
- Mapping local optical densities of states in silicon photonic structures with nanoscale electron spectroscopy
- Bridging nano-optics and condensed matter formalisms in a unified description of inelastic scattering of relativistic electron beams
- Transformation optics: a time- and frequency-domain analysis of electron-energy loss spectroscopy
- Near-field properties of plasmonic nanostructures with high aspect ratio
- The importance of substrates for the visibility of "dark" plasmonic modes
- Optical Polarization Analogs in Inelastic Free Electron Scattering
- Far-field e-beam detection of hybrid cavity-plasmonic modes in gold micro-holes
- Manipulating Acoustic and Plasmonic Modes in Gold Nanostars
- A near-field study on the transition from localized to propagating plasmons on 2D nano-wedges
- Selective probing of longitudinal and transverse plasmon modes with electron phase-matching
- Plasmon-interband hybridization and anomalous production of hot electrons in aluminum nanoantennas
- Electron-beam induced emergence of mesoscopic ordering in layered MnPS
- Electron and Light Induced Stimulated Raman Spectroscopy for Nanoscale Molecular Mapping
- Analytical solutions to zeroth-order dispersion relations of a cylindrical metallic nanowire
- Quantum interaction of sub-relativistic aloof electrons with mesoscopic samples
- Spatio-spectral metrics in electron energy loss spectroscopy as a tool to resolve nearly degenerate plasmon modes in dimer plasmonic antennas
- Imaging of Antiferroelectric Dark Modes in an Inverted Plasmonic Lattice
- Tomographic reconstruction of quasistatic surface polariton fields
- Electron energy-loss spectroscopy on freestanding perforated gold films
- Real-time surface plasmon polariton propagation in silver nanowires
- Independent engineering of individual plasmon modes in plasmonic dimers with conductive and capacitive coupling
- Imaging of plasmonic modes of silver nanoparticles using high-resolution cathodoluminescence spectroscopy